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The effect of surface pattern property on the advancing motion of three-dimensional droplets
1. | School of Mathematics and Statistics, Guangxi Normal University, Guilin 541004, China |
2. | School of Mathematical Sciences, Guizhou Normal University, Guiyang 550025, China |
3. | Computational Transport Phenomena Laboratory, King Abdullah University of Science and Technology, Thuwal 23955-6900, Saudi Arabia |
We investigate numerically the advancing motion of 3D droplets spreading on physically flat chemically heterogeneous surfaces with periodic structures. We use the Navier-Stokes-Cahn-Hilliard equations with the generalized Navier boundary conditions to model the motion of droplets. Based on a convex splitting scheme, we have done numerical simulations and compared the results between different surface patterns quantitatively. We study the effect of pattern property on the advancing motion of three phase contact lines, the critical volume at the contact line jump and the effective advancing angles. By increasing the volume of droplet slowly on heterogeneous surfaces with different pattern property, we find that the advancing contact line approaches an equiangular octagon for the patterned surface with periodic squares separated by channels and approaches a regular hexagon for the patterned surface with periodic circles in regular hexagonal arrays. The shape of three-phase contact line is much more determined by the macro structure of the pattern than the micro structure of the pattern in each period.
References:
[1] |
S. Brandon, N. Haimovich, E. Yeger and A. Marmur, Partial wetting of chemically patterned surfaces: The effect of drop size, J. Colloid Interf. Sci., 263 (2003), 237-243. Google Scholar |
[2] |
S. Brandon and A. Marmur, Simulation of contact angle hysteresis on chemically heterogeneous surfaces, J. Colloid Interf. Sci., 183 (1996), 351-355. Google Scholar |
[3] |
S. Brandon, A. Wachs and A. Marmur, Simulated contact angle hysteresis of a three-dimensional drop on a chemically heterogeneous surface: A numerical example, J. Colloid Interf. Sci., 191 (1997), 110-116. Google Scholar |
[4] |
A. B. D. Cassie and S. Baxter,
Wettability of porous surfaces, Trans. Faraday Soc., 40 (1944), 546-551.
doi: 10.1039/tf9444000546. |
[5] |
D. Chatain, D. Lewis, J.-P. Baland and W. C. Carter,
Numerical analysis of the shapes and energies of droplets on micropatterned substrates, Langmuir, 22 (2006), 4237-4243.
doi: 10.1021/la053146q. |
[6] |
P. G. de Gennes,
Wetting: Statics and dynamics, Rev. Mod. Phys., 57 (1985), 827-863.
doi: 10.1103/RevModPhys.57.827. |
[7] |
M. Gao and X.-P. Wang,
A gradient stable scheme for a phase field model for the moving contact line problem, J. Comput. Phys., 231 (2012), 1372-1386.
doi: 10.1016/j.jcp.2011.10.015. |
[8] |
H. Gouin,
The wetting problem of fluids on solid surfaces. Ⅰ. The dynamics of contact lines, Contin. Mech. Thermodyn., 15 (2003), 581-596.
doi: 10.1007/s00161-003-0136-2. |
[9] |
H. Gouin,
The wetting problem of fluids on solid surfaces. Ⅱ. The contact angle hysteresis, Contin. Mech. Thermodyn., 15 (2003), 597-611.
doi: 10.1007/s00161-003-0137-1. |
[10] |
M. Iwamatsu,
Contact angle hysteresis of cylindrical drops on chemically heterogeneous striped surfaces, J. Colloid Interf. Sci., 297 (2006), 772-777.
doi: 10.1016/j.jcis.2005.11.032. |
[11] |
J. F. Joanny and P. G. de Gennes,
A model for contact angle hysteresis, J. Chem. Phys., 81 (1984), 552-562.
doi: 10.1142/9789812564849_0048. |
[12] |
R. E. Johnson and R. H. Dettre,
Contact-angle hysteresis. 3. study of an idealized heterogeneous surface, J. Phys. Chem., 68 (1964), 1744-1749.
doi: 10.1021/j100789a012. |
[13] |
H. Kusumaatmaja and J. M. Yeomans,
Modeling contact angle hysteresis on chemically patterned and superhydrophobic surfaces, Langmuir, 23 (2007), 6019-6032.
doi: 10.1021/la063218t. |
[14] |
S. T. Larsen and R. Taboryski,
A Cassie-like law using triple phase boundary line fractions for faceted droplets on chemically heterogeneous surfaces, Langmuir, 25 (2009), 1282-1284.
doi: 10.1021/la8030045. |
[15] |
L. Luo, X.-P. Wang and X.-C. Cai,
An efficient finite element method for simulation of droplet spreading on a topologically rough surface, J. Comput. Phys., 349 (2017), 233-252.
doi: 10.1016/j.jcp.2017.08.010. |
[16] |
A. Marmur,
Contact-angle hysteresis on heterogeneous smooth surfaces, J. Colloid Interf. Sci., 168 (1994), 40-46.
doi: 10.1006/jcis.1994.1391. |
[17] |
T. Qian, X. P. Wang and P. Sheng, Molecular scale contact line hydrodynamics of immiscible flows, Phys. Rev. E, 68 (2003), 016306.
doi: 10.1103/PhysRevE.68.016306. |
[18] |
W. Ren,
Wetting transition on patterned surfaces: Transition states and energy barriers, Langmuir, 30 (2014), 2879-2885.
doi: 10.1021/la404518q. |
[19] |
L. W. Schwartz and S. Garoff,
Contact angle hysteresis on heterogeneous surfaces, Langmuir, 1 (1985), 219-230.
doi: 10.1021/la00062a007. |
[20] |
L. W. Schwartz and S. Garoff,
Contact angle hysteresis and the shape of the 3-phase line, J. Colloid Interf. Sci., 106 (1985), 422-437.
doi: 10.1016/S0021-9797(85)80016-3. |
[21] |
P. S. Swain and R. Lipowsky,
Contact angles on heterogeneous surfaces: A new look at Cassie's and Wenzel's laws, Langmuir, 14 (1998), 6772-6780.
doi: 10.1021/la980602k. |
[22] |
X.-P. Wang, T. Qian and P. Sheng,
Moving contact line on chemically patterned surfaces, J. Fluid Mech., 605 (2008), 59-78.
doi: 10.1017/S0022112008001456. |
[23] |
R. N. Wenzel,
Resistance of solid surfaces to wetting by water, Ind. Eng. Chem., 28 (1936), 988-994.
doi: 10.1021/ie50320a024. |
[24] |
G. Wolansky and A. Marmur,
The actual contact angle on a heterogeneous rough surface in three dimensions, Langmuir, 14 (1998), 5292-5297.
doi: 10.1021/la960723p. |
[25] |
X. Xu,
Analysis for wetting on rough surfaces by a three-dimensional phase field model, Discrete Contin. Dyn. Syst. Ser. B, 21 (2016), 2839-2850.
doi: 10.3934/dcdsb.2016075. |
[26] |
X. Xu and X. Wang,
Analysis of wetting and contact angle hysteresis on chemically patterned surfaces, SIAM J. Appl. Math., 71 (2011), 1753-1779.
doi: 10.1137/110829593. |
[27] |
T. Young,
An essay on the cohesion of fluids, Philos. Trans. R. Soc. London, 95 (1805), 65-87.
doi: 10.1098/rstl.1805.0005. |
[28] |
H. Zhong, X.-P. Wang, A. Salama and S. Sun,
Quasistatic analysis on configuration of two-phase flow in Y-shaped tubes, Comput. Math. Appl., 68 (2014), 1905-1914.
doi: 10.1016/j.camwa.2014.10.004. |
[29] |
H. Zhong, X.-P. Wang and S. Sun,
A numerical study of three-dimensional droplets spreading on chemically patterned surfaces, Discrete Contin. Dyn. Syst. Ser. B, 21 (2016), 2905-2926.
doi: 10.3934/dcdsb.2016079. |
show all references
References:
[1] |
S. Brandon, N. Haimovich, E. Yeger and A. Marmur, Partial wetting of chemically patterned surfaces: The effect of drop size, J. Colloid Interf. Sci., 263 (2003), 237-243. Google Scholar |
[2] |
S. Brandon and A. Marmur, Simulation of contact angle hysteresis on chemically heterogeneous surfaces, J. Colloid Interf. Sci., 183 (1996), 351-355. Google Scholar |
[3] |
S. Brandon, A. Wachs and A. Marmur, Simulated contact angle hysteresis of a three-dimensional drop on a chemically heterogeneous surface: A numerical example, J. Colloid Interf. Sci., 191 (1997), 110-116. Google Scholar |
[4] |
A. B. D. Cassie and S. Baxter,
Wettability of porous surfaces, Trans. Faraday Soc., 40 (1944), 546-551.
doi: 10.1039/tf9444000546. |
[5] |
D. Chatain, D. Lewis, J.-P. Baland and W. C. Carter,
Numerical analysis of the shapes and energies of droplets on micropatterned substrates, Langmuir, 22 (2006), 4237-4243.
doi: 10.1021/la053146q. |
[6] |
P. G. de Gennes,
Wetting: Statics and dynamics, Rev. Mod. Phys., 57 (1985), 827-863.
doi: 10.1103/RevModPhys.57.827. |
[7] |
M. Gao and X.-P. Wang,
A gradient stable scheme for a phase field model for the moving contact line problem, J. Comput. Phys., 231 (2012), 1372-1386.
doi: 10.1016/j.jcp.2011.10.015. |
[8] |
H. Gouin,
The wetting problem of fluids on solid surfaces. Ⅰ. The dynamics of contact lines, Contin. Mech. Thermodyn., 15 (2003), 581-596.
doi: 10.1007/s00161-003-0136-2. |
[9] |
H. Gouin,
The wetting problem of fluids on solid surfaces. Ⅱ. The contact angle hysteresis, Contin. Mech. Thermodyn., 15 (2003), 597-611.
doi: 10.1007/s00161-003-0137-1. |
[10] |
M. Iwamatsu,
Contact angle hysteresis of cylindrical drops on chemically heterogeneous striped surfaces, J. Colloid Interf. Sci., 297 (2006), 772-777.
doi: 10.1016/j.jcis.2005.11.032. |
[11] |
J. F. Joanny and P. G. de Gennes,
A model for contact angle hysteresis, J. Chem. Phys., 81 (1984), 552-562.
doi: 10.1142/9789812564849_0048. |
[12] |
R. E. Johnson and R. H. Dettre,
Contact-angle hysteresis. 3. study of an idealized heterogeneous surface, J. Phys. Chem., 68 (1964), 1744-1749.
doi: 10.1021/j100789a012. |
[13] |
H. Kusumaatmaja and J. M. Yeomans,
Modeling contact angle hysteresis on chemically patterned and superhydrophobic surfaces, Langmuir, 23 (2007), 6019-6032.
doi: 10.1021/la063218t. |
[14] |
S. T. Larsen and R. Taboryski,
A Cassie-like law using triple phase boundary line fractions for faceted droplets on chemically heterogeneous surfaces, Langmuir, 25 (2009), 1282-1284.
doi: 10.1021/la8030045. |
[15] |
L. Luo, X.-P. Wang and X.-C. Cai,
An efficient finite element method for simulation of droplet spreading on a topologically rough surface, J. Comput. Phys., 349 (2017), 233-252.
doi: 10.1016/j.jcp.2017.08.010. |
[16] |
A. Marmur,
Contact-angle hysteresis on heterogeneous smooth surfaces, J. Colloid Interf. Sci., 168 (1994), 40-46.
doi: 10.1006/jcis.1994.1391. |
[17] |
T. Qian, X. P. Wang and P. Sheng, Molecular scale contact line hydrodynamics of immiscible flows, Phys. Rev. E, 68 (2003), 016306.
doi: 10.1103/PhysRevE.68.016306. |
[18] |
W. Ren,
Wetting transition on patterned surfaces: Transition states and energy barriers, Langmuir, 30 (2014), 2879-2885.
doi: 10.1021/la404518q. |
[19] |
L. W. Schwartz and S. Garoff,
Contact angle hysteresis on heterogeneous surfaces, Langmuir, 1 (1985), 219-230.
doi: 10.1021/la00062a007. |
[20] |
L. W. Schwartz and S. Garoff,
Contact angle hysteresis and the shape of the 3-phase line, J. Colloid Interf. Sci., 106 (1985), 422-437.
doi: 10.1016/S0021-9797(85)80016-3. |
[21] |
P. S. Swain and R. Lipowsky,
Contact angles on heterogeneous surfaces: A new look at Cassie's and Wenzel's laws, Langmuir, 14 (1998), 6772-6780.
doi: 10.1021/la980602k. |
[22] |
X.-P. Wang, T. Qian and P. Sheng,
Moving contact line on chemically patterned surfaces, J. Fluid Mech., 605 (2008), 59-78.
doi: 10.1017/S0022112008001456. |
[23] |
R. N. Wenzel,
Resistance of solid surfaces to wetting by water, Ind. Eng. Chem., 28 (1936), 988-994.
doi: 10.1021/ie50320a024. |
[24] |
G. Wolansky and A. Marmur,
The actual contact angle on a heterogeneous rough surface in three dimensions, Langmuir, 14 (1998), 5292-5297.
doi: 10.1021/la960723p. |
[25] |
X. Xu,
Analysis for wetting on rough surfaces by a three-dimensional phase field model, Discrete Contin. Dyn. Syst. Ser. B, 21 (2016), 2839-2850.
doi: 10.3934/dcdsb.2016075. |
[26] |
X. Xu and X. Wang,
Analysis of wetting and contact angle hysteresis on chemically patterned surfaces, SIAM J. Appl. Math., 71 (2011), 1753-1779.
doi: 10.1137/110829593. |
[27] |
T. Young,
An essay on the cohesion of fluids, Philos. Trans. R. Soc. London, 95 (1805), 65-87.
doi: 10.1098/rstl.1805.0005. |
[28] |
H. Zhong, X.-P. Wang, A. Salama and S. Sun,
Quasistatic analysis on configuration of two-phase flow in Y-shaped tubes, Comput. Math. Appl., 68 (2014), 1905-1914.
doi: 10.1016/j.camwa.2014.10.004. |
[29] |
H. Zhong, X.-P. Wang and S. Sun,
A numerical study of three-dimensional droplets spreading on chemically patterned surfaces, Discrete Contin. Dyn. Syst. Ser. B, 21 (2016), 2905-2926.
doi: 10.3934/dcdsb.2016079. |









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